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41.
A. Gelencsér A. Hoffer G. Kiss E. Tombácz R. Kurdi L. Bencze 《Journal of Atmospheric Chemistry》2003,45(1):25-33
Current climate models seem to underestimate the flux of solar energy absorbed by the global troposphere. All of these models are constrained with the assumption that cloud droplets consist of pure water. Here we demonstrate in a simple laboratory experiment that aromatic hydroxy-acids which are found in continental fine aerosol can react with hydroxyl radicals under typical conditions prevalent in cloud water influenced by biomass burning. The reactions yield colored organic species which do absorb solar radiation. We also suggest that the products of such reactions may be humic-like substances whose presence in continental aerosol has been confirmed but their source mechanisms are still much sought after. We also attempt to give a first order estimate of the enhancement of water absorption at a visible wavelength under atmospheric conditions. 相似文献
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The effect of elevated nitric acid concentrations on cloud particle number concentrations and sizes of mixed phase cirrus cloud (containing both supercooled liquid and frozen ice particles) is studied using a detailed multicomponent condensation model. Our model calculations suggest that high nitric acid volume mixing ratios (VMRs), corresponding to upper tropospheric measurements, can increase the ice crystal number concentrations substantially especially in the case of freezing of non-activated solution droplets (as opposed to freezing of supercooled cloud droplets). This is due to increased droplet sizes caused by nitric acid absorption and the resulting uptake of water. 相似文献
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Observations show that the sequences of microsecond-scale pulses are produced in cloud flashdischarge processes.In the present work we report on measurements of larger bipolar pulses(LBP)of the radiation fields which are classified into four types according to their waveshapes andpolarities of initial peak.Either positive or negative pulse contains two kinds of waveshapes:onewith a smooth rise and the other with 2 or 3 fast-rising pulse superimposed on the initial half cycle.The pulse waveshape characteristics in both time and frequency domains are as follows.Among2908 samples there are 45% of the positive polarity and 55% of the negative polarity.The positivepulses tend to have distinctly smaller values than negative pulses in rise time,half width and zero-crossing time of the initial peak.The peaks of positive pulse spectra tend to occur at a higherfrequency than those of negative pulses.Despite differences above,positive and negative pulseshave a similar total duration. 相似文献
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利用热带天气图,日本GMS卫星云图,ECMWF格点风场资料,对澳大利亚东南部持续性降水的两类主要天气过程,热带云涌-冷锋尾流气旋锋生过程和阻塞反气旋北侧回流降水过程进行了分析,从云型演变,环流形热,热带流场等方面揭示了澳大利亚东南部持续性降水天气过程的基本特征、为业务预报提供参考。 相似文献